)-thioether-functionalised NHC ligands. Yi Huang, Xiaodan Chong, Cuibo Liu, Yu Liang, Bin Zhang. Redox Isomerization/Acceptorless Dehydrogenation. Aerobic dehydrogenation of amines to nitriles catalyzed by triazolylidene ruthenium complexes with O Complexes upon Deprotonation and Their Application in Catalytic Carbene Carbonylation Reactions. and Ir -based catalysts via sustainable aerobic oxidation. Satoshi Muratsugu, Sutasinee Kityakarn, Fei Wang, Nozomu Ishiguro, Takashi Kamachi, Kazunari Yoshizawa, Oki Sekizawa, Tomoya Uruga, Mizuki Tada. Marta Olivares, Pascal Knörr, Martin Albrecht. 4 Electronic Supporting Information files are available without a subscription to ACS Web Editions. Nitrogen-coordinated cobalt nanocrystals for oxidative dehydrogenation and hydrogenation of N-heterocycles. Au This article is cited by Zan Chen, Quan Zhou, Qiao‐Lin Wang, Pu Chen, Bi‐Quan Xiong, Yun Liang, Ke‐Wen Tang, Yu Liu. Iron‐Mediated Cyanoalkylsulfonylation/Arylation of Active Alkenes with Cycloketone Oxime Derivatives via Sulfur Dioxide Insertion. Article Views are the COUNTER-compliant sum of full text article downloads since November 2008 (both PDF and HTML) across all institutions and individuals. Easy Ruthenium‐Catalysed Oxidation of Primary Amines to Nitriles under Oxidant‐Free Conditions. Information about how to use the RightsLink permission system can be found at Please reconnect. Recent Advances in the Synthesis of Aryl Nitrile Compounds. Mengdi Zhao, Wei Zhang, and Zengming Shen .

Gibbon, Benjamin Gabriele, Mikhail Malanin, Klaus-Jochen Eichhorn. Catalytic oxidations by dehydrogenation of alkanes, alcohols and amines with defined (non)-noble metal pincer complexes.

Dinesh Talwar, Angela Gonzalez-de-Castro, Ho Yin Li, Jianliang Xiao. Wandi Zhang, Christopher W. Haskins, Yang Yang, Mingji Dai. Chidambaram Gunanathan and David Milstein . without permission from the American Chemical Society. Users are Iridium Half-Sandwich Complexes with Di- and Tridentate Bis(pyridylimino)isoindolato Ligands: Stoichiometric and Catalytic Reactivity. Users are the Altmetric Attention Score and how the score is calculated. Acetonitrile as a Cyanating Reagent: Cu-Catalyzed Cyanation of Arenes. (111) facets. ChemInform Abstract: Oxidant-Free Conversion of Primary Amines to Nitriles.. Yo Han Kim, Seung Kyu Hwang, Yoon Sik Lee, Jung Won Kim. Hydrogen Transfer Catalysis beyond the Primary Coordination Sphere. Direct synthesis of nitriles from cleavage of C C double bond with nitrite as the nitrogen source and oxidant. not otherwise permitted to reproduce, republish, redistribute, or sell any Supporting Information E-mail: You’ve supercharged your research process with ACS and Mendeley! You have to login with your ACS ID befor you can login with your Mendeley account. Hirotaka Nagao, Naoto Shimura, Haruka Yonezawa. 2 Stereoretentive Deuteration of α-Chiral Amines with D2O. Zhou Tang, Cristina Tejel, Marc Martinez de Sarasa Buchaca, Martin Lutz, Jarl Ivar van der Vlugt, Bas de Bruin. 1 Bis(pyridylimino)isoindolato (BPI) Osmium Complexes: Structural Chemistry and Reactivity. A Journey from Thermally Tunable Synthesis to Spectroscopy of Phenylmethanimine in Gas Phase and Solution. Files available from the ACS website may be downloaded for personal use only. O Hydrogen pressure influences the selectivity for the primary amines. Sondomoyee K. Moromi, S.M.A. o Selective Acceptorless Dehydrogenation of Primary Amines to Imines by Core–Shell Cobalt Nanoparticles. Find more information on the Altmetric Attention Score and how the score is calculated. Susanta Hazra, Ekta Malik, Abhishek Nair, Vikas Tiwari, Pritam Dolui, Anil J. Elias.
Nitriles can be converted to 1° amines by reaction with LiAlH 4. 2 The unprecedented strategy of the oxidation of an amine directly to a nitrile oxide was used in this cyclization process. Efficient Oxidative Dehydrogenation of N-Heterocycles over Nitrogen-Doped Carbon-Supported Cobalt Nanoparticles. Please reconnect. -Aminobenzamides and Allylic Alcohols to Quinazolinones ) complex. -Quinone Methides Generated from 2-(1-Tosylalkyl)phenols. Qiang Liu, Bao Fang, Xiaohui Bai, Yuan Liu, Yao Wu, Guiming Xu, Cancheng Guo. Information. Citations are the number of other articles citing this article, calculated by Crossref and updated daily. S Primary amines contain the -NH 2 group. Bond Activation and Catalysis by Ruthenium Pincer Complexes.

Reductive C−C Coupling from α,β‐Unsaturated Nitriles by Intercepting Keteniminates. Carbohydrate-Functionalized 1,2,3-Triazolylidene Complexes for Application in Base-Free Alcohol and Amine Oxidation. N Pyridyl-substituted mesoionic triazolylidene ruthenium cymene complexes catalyze the oxidation of both aromatic and aliphatic amines to nitriles with high activity and selectivity under benign conditions using dioxygen as the terminal oxidant.
Control experiments support a nitrile oxide intermediate mechanism for this novel class of oxidative cyclization reactions. An amide-derived NNN-Ru(II) hydride complex catalyzes oxidant-free, acceptorless, and chemoselective dehydrogenation of primary and secondary amines to the corresponding nitriles and imines with liberation of dihydrogen. Please note: If you switch to a different device, you may be asked to login again with only your ACS ID. Modular Attachment of Appended Boron Lewis Acids to a Ruthenium Pincer Catalyst: Metal–Ligand Cooperativity Enables Selective Alkyne Hydrogenation. redistribute this material, requesters must process their own requests via the RightsLink permission Find more information about Crossref citation counts. Xinjiang Cui, Yuehui Li, Stephan Bachmann, Michelangelo Scalone, Annette-Enrica Surkus, Kathrin Junge, Christoph Topf, and Matthias Beller . Synthesis and Characterization of Iron–Nitrogen-Doped Graphene/Core–Shell Catalysts: Efficient Oxidative Dehydrogenation of N-Heterocycles. Examining the early stages of thermal oxidative degradation in epoxy-amine resins. For permission to reproduce, republish and John-Paul J. Lillian V. A. Hale and Nathaniel K. Szymczak . Pei Chen, Qian-Qian Zhang, Jia Guo, Lu-Lu Chen, Yan-Bo Wang, Xiao Zhang. About. Departement für Chemie und Biochemie, Universität Bern, Freiestrasse 3, CH-3012 Bern, Switzerland redistribute this material, requesters must process their own requests via the RightsLink permission Yamin Zhu, Mengdi Zhao, Wenkui Lu, Linyi Li, and Zengming Shen . Direct C–H Cyanoalkylation of Heteroaromatic N-Oxides and Quinones via C–C Bond Cleavage of Cyclobutanone Oximes. Article Views are the COUNTER-compliant sum of full text article downloads since November 2008 (both PDF and HTML) across all institutions and individuals. Thierry Achard, Julien Egly, Michel Sigrist, Aline Maisse‐François, Stéphane Bellemin‐Laponnaz. reduction catalysis. A Proton-Switchable Bifunctional Ruthenium Complex That Catalyzes Nitrile Hydroboration. Alessio Melli, Simone Potenti, Mattia Melosso, Sven Herbers, Lorenzo Spada, Andrea Gualandi, Kevin G. Lengsfeld, Luca Dore, Philipp Buschmann, Pier Giorgio Cozzi, Jens‐Uwe Grabow, Vincenzo Barone, Cristina Puzzarini. The nitrile reacts with the lithium tetrahydridoaluminate in solution in ethoxyethane (diethyl ether, or just "ether") followed by treatment of the product of that reaction with a dilute acid. Cu-Catalyzed Cyanation of Indoles with Acetonitrile as a Cyano Source. Get article recommendations from ACS based on references in your Mendeley library. Weiguang Chen, Julien Egly, Amalia I. Poblador-Bahamonde, Aline Maisse-Francois, Stéphane Bellemin-Laponnaz, Thierry Achard. A facile oxidative heterocyclization of commercially available amines and tert-butyl nitrite with alkynes or alkenes leading to isoxazoles or isoxazolines is described.

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